June 2012 Issue - Volume 8, Number 3

Fukushima Daiichi

Takashi Murakami and Rodney C. Ewing – Guest Editors

Table of Contents

Thematic Articles

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This thematic issue of Elements describes the events at the Fukushima Daiichi nuclear power plant on March 11, 2011, and the aftermath.
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Rapid seismological analyses, carried out within minutes of the March 11, 2011, Tohoku earthquake, were crucial in providing an earthquake ground shaking and tsunami early warning and in hastening the evacuation of the population along Japan’s northeastern coast. By 20 to 30 minutes after fault rupture began, these analyses had established that the event had a moment magnitude of Mw = 9 and involved shallow thrust faulting on the plate boundary megathrust. Preparation for future large earthquakes on megathrusts in Japan and elsewhere should include onshore and offshore geodetic monitoring of strain accumulation, implementation of rapid earthquake and tsunami warning systems, and public training and education for shaking and tsunami response.
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The major nuclear accident at the Fukushima Daiichi nuclear power plant more than one year ago was the result of a combination of four interrelated factors: site selection, external hazard assessment and site preparation, the utility’s approach to risk management, and fundamental reactor design. The reactor accident was initiated by a magnitude 9 earthquake, followed by an even more damaging tsunami. An insufficient tsunami defense-in-depth strategy led to significant core damage in three units and radioactive release to the environment. This paper provides a summary of the sequence of events that led to the accident and current efforts to contain and manage the released radioactivity.
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On March 11, 2011, an earthquake and tsunami hit the northeast coast of Japan and damaged the Fukushima Daiichi nuclear power plant, leading to the release of radioactive material into the atmosphere. We trace the evolution of radioactivity release to the atmosphere and subsequent dispersion as simulated by models, and we compare these to actual measurements. Four main release periods are highlighted. The first event had limited consequences to the north of the power plant along the coast; the second had no impact on Japanese territory because the plumes travelled toward the Pacific Ocean; the third was responsible for significant and longterm impact, especially northwest of the plant; and the last had consequences of lesser impact on the Tokyo area.
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Radionuclides, such as 134Cs, 137Cs, and 131I, were released during the Fukushima Daiichi nuclear power plant accident in March 2011. Their distribution was monitored by airborne surveys and soil sampling. The most highly contaminated areas are to the northwest of the plant and in the Naka-dori region of Fukushima Prefecture; this contamination was mainly the result of wet deposition on March 15. Radionuclides were also released on March 21, and they were dispersed up to 200 km south of the plant. The Cs/I ratios are different for these two events, probably because of differences in the initial ratios in the airborne plumes and the amount of wet deposition. Numerical simulations of the dispersion process and vertical profiles of radionuclides in soils are used to describe the contamination of soils.
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Five models have been used to estimate the oceanic dispersion of 137Cs from the Fukushima Daiichi nuclear power plant during March and April 2011, following the accident on March 11, 2011. The total discharged activity of 137Cs is estimated to be 2 to 15 petabequerels. A weak southward current along the Fukushima coast was responsible for the initial transport direction, while mesoscale eddy-like structures and surface-current systems contributed to dispersion in areas beyond the continental shelf. Most of the discrepancies among the models in April are caused by differences in how the mesoscale current structures off the Ibaraki coast are represented.
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Used nuclear fuel is a redox-sensitive semiconductor consisting of uranium dioxide containing a few percent of fission products and up to about one percent transuranium elements, mainly plutonium. The rapid increase in temperature in the cores of the Fukushima reactors was caused by the loss of coolant in the aftermath of the damage from the tsunami. Temperatures probably well above 2000°C caused melting of not only the UO2 in the fuel but also the zircaloy cladding and steel, forming a quenched melt, termed corium. Substantial amounts of volatile fission products, such as Cs and I, were released during melting, but the less volatile fission products and the actinides (probably >99.9%) were incorporated into the corium as the melt cooled and was quenched. The corium still contains these radionuclides, which leads to a very large long-term radiotoxicity of the molten reactor core. The challenge for environmental scientists is to assess the longterm interactions between water and the mixture of corium and potentially still-existing unmelted fuel, particularly if the molten reactor core is left in place and covered with a sarcophagus for hundreds of years. Part of the answer to this question can be found in the knowledge that has been gained from research into the disposal of spent nuclear fuel in a geologic repository.
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